Even cheap PC2700 should be able to do at least 166 at 1:1 and CAS 2.5. Bumping the memory voltage up is usually good for some extra speed, just don't overdo it. Have you tried changing the ratio manually? You'll need to set SPD (Serial Presence Detect) to off in the BIOS.
I'm no expert with Nforce chipset motherboards. You'd probably be able to find more information on memory settings for your board in the Abit AMD motherboards subforum, or the storage and memory subforum.