I'm not sure where multi's are at nowadays, but I'll give you my procedure on dialing in a chip:
I start off making sure the unlock is good by setting fsb low and checking all the multis; then I up the multi with 100mhz fsb and see how high it can go stable- use some fsb if you run out of multipliers.
Step two: drop to a low multi and increase fsb until it won't boot- then back off until its stable.
Now you know two things: how fast the chip can go, and how high you can jack the bus speed. Find the best compromise. leaning towards as high a bus as possible.
I start off with voltages and memory timing at defaults, then once the oc is set I'll start tweaking voltage and ram for a bit more.
Gotta bench at every setting at this point to really know for sure what settings will get the best results so it takes a long time- I put a week or two into really doing it right with a new system.
And when I have everything figured out I do a clean os install, since by now it should be pretty trashed
