It's pretty simple. Firsly, go to
www.tweakfiles.com, and get nvMax (Or RivaTuner, but I prefere nvMax).
Make sure you have the latest drivers.
Start overclocking. Turn up the core 2 MHz. Test the settings in Unreal Tournament, or Quake 3, or any "new" 3D game. (Look for white spots;snow [AKA Artifacts])
If there are no artifacts, try another 2 MHz. Chances are you'll get up between 10 and 20 MHz. (Don't jump all the way up though)
When you find a clock speed that doesn't have (or has very little) artifacts, set the clock speed down 2 or 3 MHz. There's your core speed.
Do the same with the memory. Up 2 MHz, test, up 2 MHz, test, etc., find minor artifacts, set it down 2-3MHz.
Simple, eh? I hope you can get at least another 15 MHz out of both memory and core speed! (If you have problems after turning up the speeds, I.E., constant system hangs, page faults, and what not, then you'll probably need to affix a larger heatsink to the GPU to solve heat issues, which cause problems. There are plenty of articles on how to do that right.)