Depends on how far you want to go. Generally those who want to push it as far as it will go, will push it until they see minor artifacting, and then dial it back some and benchmark it for many hours to prove it's stability. 69c is very cool for those speeds, are you sure that's on full load? Keep in mind that after you close the benchmark, your GPU temp will drop IMMEDIATELY. Before you can even get to the temp monitor after ending the benchmark, it's probably dropped quite a bit (5-15c). Get your hands on ATI Tool and pop open the spinning 3D image, and watch your temps rise until it reaches peak.
Keep an eye out for artifacts. If you see anything funky dial it back and benchmark it agin. My rule of thumb is that if I can game for 3 hours straight without any issues whatsoever, then it's stable. Other people will bench for shorter or longer. Just be careful and conservative. IMO that is a darn good OC you have right now. Whether or not you can go higher, I dunno. I'm not comlpetely familiar with these cards yet. I'm sure others will chime in and help you more than I can. Good luck.