OC'ing
Welcome to the forums!
You can find your card's limit by benchmarking it at new settings. First, disable v-sync in display properties/advanced/direct3d. If it locks up, reboots, or exits 3dmark2001, then the GPU is probably clocked too high. If you see sparkly dots and distortions on the screen when benchmarking, then the memory is probably clocked too high. Test core speed and memory seperately first and find the limit of each. Then try raising both at the same time and go as high as you can. Note: without good cooling, I wouldn't raise either setting more than 10%, well maybe the memory could go higher than 10%. And watch the 3dmark scores, sometimes it works at a higher setting, but gets a lower score. Make sure you close any unnecessary programs before benchmarking. And you might want to try a different program for tweaking the card. I used Winfox for a while, but I got better results with NVmax. There's also Riva Tuner, Powerstrip, and a few others. Changing your drivers will give you better performance, too, but it may disable your TV-out.
When you've found the right settings for your card, loop the benchmark 10 or 20 times, or play some games for an hour or two. I fyou have problems, lower the settings.
Hope this general info helps you. Have questions? Will answer.