First, I'm going to assume you meant SRT (smart response technology aka ssd caching).
I used SRT for a while to accelerate my games hard drive (raptor, 600gb) so it wasn't my boot drive, I had a dedicated 240gb SSD for that. But the raid array SRT creates crashed a few times and I had to recheck my steam cache, it ended up redownloading over 80% of my games because of corrupted files. That's when I disabled SRT.
If it works, great. But when it starts having problems, it can be a nightmare.
Honestly I'd suggest you save some cash and get a decent sized SSD (120+) for your boot drive and move everything that doesn't need to be on it (user folder, non-critical software, etc.) on a regular hard drive to leave enough room for your important stuff (windows, a few main games, software you want to open fast like possibly your office suite, etc.). I know you currently have a 60gb SSD, you can still use that for other important applications too.