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This is the same for me, as well. I remember reading about that build and was in absolute amazement.It was guys like you and articles like that which got me hooked here before I ever registered. You are an OG OCFer.
If I wanted to go sub-ambient, I'd just go with a phase change unit.
I recall toothpaste doing fairly well also.
Now, is a 140mm radiator that much better than a 120mm rad?
Quick Ancient History Lesson: My first computer was a 4 Megahertz Radio Shack TRS-80 Model III. This was back when Jobs and Wozniack were selling their brand new Apple. This was at least 2 or 3 years before the first IBM desktop unit (called the Acorn) was even released. I bought my old Model III around 1980.
A good compromise on this is getting a 140mm to 120mm adapter and putting a 120mm fan on your 140mm rad.
I've got this! It depends how you mean, if you mean does it offer better maximum performance, then yes, I'd say 140mm rads are better, that extra 400mm^2 of space is pretty significant and testing confirms this. The issue with 140mm rads is that the fan selection for them is attrocious, especially in comparison to what is available for 120mm radiators. There are no thick 140mm fans, and almost every 140mm fan out there runs on a motor that was (presumably) designed for a 120mm fan, which means 1 major thing: lack of static pressure. Because of this, the gap between 140mm and 120mm rads is actually not as large as it should be. A good compromise on this is getting a 140mm to 120mm adapter and putting a 120mm fan on your 120mm rad. The downside to this is that you'll not be seeing the performance you would with a 140mm fan, were there fans that were sensibly designed in that size.
I recall toothpaste doing fairly well also.