So you had the CPU/NB at 2600 at one point, correct? And at that point your HT Link was only 2000, correct. It may help to bump the HT Link up to say 2400 as the Thubans don't like a wide differential between the CPU/NB and the HT Link.
When you tried the FSB with the overclocking did you realize that raising the FSB also raises the memory frequency, the CPU/NB frequency and the HT Link frequency at the same time? They are linked together. When you use the FSB you have to keep an eye on the other two and make adjustments if their frequencies get too high. This is where most beginner overclockers go wrong when using the FSB.
My usual approach is to lower the RAM divider one notch below what it is rated for. So if the RAM is rated for 1333 mhz I will set it ot 1066 in bios. I will also lower the CPU/NB and the HT Link to 1800 mhz. I'll give the CPU voltage a .025 bump and set the CPU/NB voltage to 1.225. All this at the front end. Then I start to increase the FSB in 5-10 mhz increments until I can't pass a 20 minute Prime95 blend test. Then I'll add a little more voltage to the CPU to get it stable again. My goal is to get the RAM back up to it's rated max frequency using the FSB only so as to make sure I'm not under utilizing my RAM. I don't touch the multiplier until I get to that point. I also keep an eye on the CPU/NB and HT Link frequencies as I raise the FSB to keep them from getting too high and causing instability. I shoot for 2500-2600 on the CPU/NB and about 2400 on the HT Link. 1.225-1.25 volts seems to be adequate most of the time to support the CPU/NB at this frequency level. After I have gotten the RAM frequency back up to snuff then I revert to the CPU multiplier if there is any overclocking room left in the CPU.