I've done this and my PC booted into Windows just now with a Multiplier of 20x.
Thus resulting in 4GHz.
How should I continue to increase the Multiplier and voltages?
Every .5x 1 step in the CPUNB upwards?
Every time you change the settings and boot into windows you need to prime for at least 20 minutes. If you make a 20 minute run, you can guess that it is fairly stable, but you will not know if it is 100% stable until you've done a 2 hour + run.
So now that you're at 4 GHZ, you need to run Prime for 20 minutes and post the results.