Don't forget your memory is rated at 2.1-2.3 volts. Stock is 1.8, so even at +.3, you were only just giving it the minimum suggested voltage for higher speeds. I would set your RAM voltage to +.4 and 1:1 multi, that way you are taking the memory out of the equation. The CPU should easily go higher..
This is assuming it's the OCZ stuff in your sig. At the bottom of their spec page, it says don't exceed 2.1v if it's listed on the module label. Is it?
http://www.ocztechnology.com/products/memory/ocz_ddr2_pc2_8500_sli_ready_edition_dual_channel