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The time to try the core unlocking would be now, before you overclock the CPU: "CPU Unlock" would need to be enabled. That's really all there is to it. Even if it seems to work at first you would need to stress test it to check for stability. To do that, download and install Prime95 and HWMonitor. Open HWMonitor on the desktop and leave it open while you run a 20 minute Prime95 "just stress testing" blend test. Watch the CPU and core temps in HWMonitor. If either begin to exceed about 65c, stop the test. The CPU temp may be expressed as a generic sensor reading in the TMPINx section of HWMonitor. If so the CPU temp would correspond to TMPIN2 since you have a Gigabyte board. CPU temp is really CPU socket temp, read from a sensor on the motherboard. Core temp is the temp of the processor itself.
If you fail the test (blue screen, lockup, spontaneous restart or one of the Prime95 core workers drops out) then try adding .025 to the CPU Voltage Control which would need to be taken off of Auto, of course. Then retest.
CPU-z reflects that you correctly changed the bios values I outlined. You are ready to start overclocking when you are done with the core unlocking experiment.
Yesterday 08:28 AM
SOMETHING ISN'T RIGHT HERE.... what CPU cooler are you using? is there TIM (thermal interface material) between the CPU/heatsink?